Title: Quantum%20Criticality%20and%20Fractionalized%20Phases.
1 Quantum Criticality and Fractionalized Phases.
- Discussion Leader G. Kotliar
- Grodon Research Conference on Correlated
Electrons 2004
2- Steve Julian overview of phase transitions in
heavy fermion systems. - Z.X. Shen ARPES Investigations of Cuprate
Superconductors. - Senthil Deconfined Criticality.
3Heavy Fermions.
- Fermi Liquid . . Correspondence between a system
of non interacting particles and the full
Hamiltonian. - High temperatures, system of moments and light
electrons. - Low temperature, heavy fermion liquid or
ordered magnet .Doniach Criteria . - In the early 80s , poster boy for Fermi Liquid
Theory.
4Late 80s early 90s Cuprate Superconductivity
Broad region of parameters where Fermi liquid
theory does not apply .
Search for new paradigms, need a starting point
to describe this phenomena.
5Heavy Fermions. 90s.
No longer a poster boy for Fermi liquid theory.
Several examples exhibiting, magnetism,
superconductivity, and their disapearence, and
regimes where Fermi liquid theory failed to give
a proper description.Megan Aronson this
morning Steve Julians talk
6Quantum Phase Transitions Standard approach
Hertz, Moriya, Millis
- Identify order parameter (s), e.g. m, D
- Write effective Lagrangian for the order
parameter. - Imaginary time is like an additional dimension.
- Carry out standard R.G, make predictions which
can be compared with experiments. - Caveat, fermions have been integrate out,
- and these are low energy degrees of freedom.
Ignore Berry phases.
7- In several materials,e.g. YbRh2Si2
experimental evidence has accumulated showing
that some AF to FL transitions ARE NOT described
by the standard approach. - Senthils talk, a new class of quantum critical
point, where degrees of freedom which are not
manifestly present in a description based on an
order parameter play a fundamental role.
8Quantum Criticality in Cupratesfrom Tallon and
Loram
Use the existence of an hypothetical or physical
quantum critical point, as a tool to approach
the physics of the cuprates . Theoretical ideas,
S. Sachdev.
9The QCP paradigm the area of influence of a
quantum critical point
10A different Approach
- The evolution of the electronic structure away
from the Mott insulating state, is key. - Need to understand this problem and the
correponding phases, before the phase
transitions. - Talk by Z.X. Shen . Photoemission studies of high
Tc. - Recent progress in understanding this problem
using cellular DMFT. )
11RVB phase diagram of the Cuprate Superconductors
- P.W. Anderson. Baskaran Zou and Anderson.
Connection between high Tc and Mott physics. - ltbgt coherence order parameter.
- K, D singlet formation order paramters.
G. Kotliar and J. Liu Phys.Rev. B 38,5412 (1988)
12- High temperature superconductivity is an
unavoidable consequence of the need to connect
with Mott insulator that does not break any
symmetries to a metallic state. - Tc decreases as the quasiparticle residue goes to
zero at half filling and as the Fermi liquid
theory is approached. - Early on, accounted for the most salient features
of the phase diagram. d-wave superconductivity,
anomalous metallic state, pseudo-gap state
13Problems with the approach.
- Numerous other competing states. Dimer phase, box
phase , staggered flux phase , Neel order, - Stability of the pseudogap state at finite
temperature. - Missing finite temperature . fluctuations of
slave bosons , - Temperature dependence of the penetration depth
Wen and Lee , Ioffe and Millis Theory - rTx-Ta x2 , Exp rT x-T a.
- Theory has uniform Z on the Fermi surface, in
contradiction with ARPES. see however Varma and
Abrahams
14Evolution of the spectral function at low
frequency.
If the k dependence of the self energy is weak,
we expect to see contour lines corresponding to
Ek const and a height increasing as we approach
the Fermi surface. Study a model of kappa
organics. Frustration.
15Evolution of the k resolved Spectral Function at
zero frequency. ( O. Parcollet G. Biroli and
GKotliar PRL, 92, 226402. (2004))
U/D2
U/D2.25
Uc2.35-.05, Tc/D1/44
16Keeps all the goodies of the slave boson mean
field and make many of the results more solid
but also removes the main difficulties.
- Can treat coherent and incoherent spectra.
- Not only superconductivity, but also the
phenomena of momentum space differentiation
(formation of hot and cold regions on the Fermi
surface) are unavoidable consequence of the
approach to the Mott insulator. - Can treat dynamical fluctuations between
different singlet order parameters. - Surprising role of the off diagonal self energy
which renormalizes t.
17Lattice and cluster self energies
18Mechanism for hot spot formation nn self energy
! General phenomena.
19Mott transition in cluster (QMC)
20- General result ? YES. Application to model with
isotropic t and t with possible relevance
cuprates M. Capone, M. Civelli, V. Kancharla, O.
Parcollet, and G.K. Switch to ED solver. See
poster by M. Civelli . - Switch of hot-cold regions in electron and hole
doped system.
21Energy Landscape of a Correlated Material and a
finite temperature approach to correlated
materials.
Energy
T
Configurational Coordinate in the space of
Hamiltonians
22(No Transcript)
23Am under pressure. Lindbaum et.al. PRB
63,2141010(2001)
24ITU J.C. Griveaux J. Rebizant G. Lander
25Overview of rho (p, T) of Am
- Note strongly increasing resistivity as f(p) at
all T. Shows that more electrons are entering the
conduction band - Superconducting at all pressure
- IVariation of rho vs. T for increasing p.
26DMFT study in the fcc structure. S. Murthy and G.
Kotliar
fcc
27LDADMFT spectra. Notice the rapid occupation of
the f7/2 band.
28One electron spectra. Experiments (Negele) and
LDADFT theory (S. Murthy and GK )
29Mott transition in open (right) and closed (left)
shell systems.
S
S
g T
Log2J1
???
Uc
S0
U
U
g 1/(Uc-U)
30- Approach the Mott transition, if the localized
configuration has an OPEN shell the mass
increases as the transition is approached. - Consistent theory, entropy increases
monotonically as U ? Uc . - Approach the Mott transition, if the localized
configuration has a CLOSED shell. We have an
apparent paradox. To approach the Mott
transitions the bands have to narrow, but the
insulator has not entropy.. SOLUTION
superconductivity intervenes.
31Mott transition in systems evolving towards a
closed shell.
- Resolution as the Mott transition is approached
from the metallic side, eventually
superconductivity intervenes to for a continuous
transition to the localized side. - DMFT study of a 2 band model for Buckminster
fullerines Capone et. al. Science ( 2002). - Mechanism is relevant to Americium.
32One dimensional Hubbard model .Compare 2 site
cluster (in exact diag with Nb8) vs exact Bethe
Anzats,V. Kancharla C. Bolech and GK PRB 67,
075110 (2003) M. CaponeM.Civelli V Kancharla
C.Castellani and GK Phys. Rev. B 69, 195105
(2004)
U/t4.
33What to do as a chair?
- Humour
- Make a connection ?
- Give a bit of orientation, for students
postdocs, historical backround. - Point of view of the relevance of quantum
critical phenomena. - Advertise a different philosophy, and approach.