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Comparison of He He to H2 H2

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Branch ratio of the ionization and dissociation; Alignment dependence for the ionization or dissociation; Branch ratio of H2 in a laser field ... – PowerPoint PPT presentation

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Title: Comparison of He He to H2 H2


1
Comparison of He/He to H2/H2
Comparison of He/He to H2/H2
2
H2 in a Laser Field
Physical Processes
  • Tunneling ionization
  • Rescattering with ionic core
  • Impact excitation
  • Field ionization and dissociation.

3
Tunneling Ionization
Effective Potential
Initial conditions
Classical trajectory
Regularized coordinates
4
Impact Excitation
5
Impact Excitation-II
6
Impact Excitation Probability
Vibration wavepacket
7
Field Ionization
?u totally ionized ?u partially ionized.
How far can proton move in one fs?
8
Field Ionization-II
9
Ionization versus Dissociation
Ionization Ei(R) V(R) V(Rj) 1/Rj 1/R
E(R) - E(Rj)
H2
Dissociation Ed(R) V(R) 0.5
Ed(R) ? Ei(R)
10
Branch Ratio
  • Total impact exication probability
  • Branch ratio of the ionization and dissociation
  • Alignment dependence for the ionization or
    dissociation
  • .

Branch ratio of H2 in a laser field
11
Ionization and Dissociation Spectra (Averaged)
12
Comparing with Experiments
H. Niikura, Nature 417 (2002) 917.
13
Ionization and Dissociation Spectra (Parallel)
14
Ionization and Dissociation Spectra(Perpendicular
)
15
Comparing with Experiments
From Lew Cockes Talk
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